This book brings together a special collection of papers on the utilization of greenhouse gases. Innovative techniques including biochemical fixation, plasma conversion, and microwave application, are a special feature of this book. The fundamental, economic, technical, and future development issues with these technologies are discussed in detail. Some novel reactor configurations and catalyst designs for the utilization of greenhouse gases are also discussed. Typically, these new reactors and catalysts represent the development of environmentally friendly chemical processes.

Preface

ix

General Overview

Carbon Dioxide Utilization: Greening Both the Energy and Chemical Industry: An Overview

2

(40)

Michele Aresta

Simultaneous Utilization

Catalysis in the Simultaneous Utilization of Greenhouse Gases

42

(15)

Zhen Yan

Hongshan Shang

Chaoxian Xiao

Yuan Kou

Novel Highly Active Reforming Catalyst System and Production of Pure H2 from CH4 and CO2 with Pd--Ag Membrane Reactor

57

(12)

Linsheng Wang

Kazuhisa Murata

Megumu Inaba

Dry Reforming of Ethane on Trimetallic Perovskites LaCoxFe1-xO3: Characterizations and Reactivity

69

(14)

G. Rodriguez

L. Bedel

A. C. Roger

L. Udron

L. Carballo

A. Kiennemann

Combined Carbon Dioxide and Steam Reforming with Methane in Low-Temperature Plasmas

83

(17)

K. Supat

S. Chavadej

L. L. Lobban

R. G. Mallinson

Influence of Electrode Configuration on Direct Methane Conversion with CO2 as a Coreactant Using Dielectric--Barrier Discharges

100

(16)

Yue-ping Zhang

Yang Li

Chang-jun Liu

Baldur Eliasson

Effect of H2S on the Reaction of CH4 with CO2 over Titania-Supported Noble Metal Catalysts

116

(14)

Andras Erdohelyi

Tamas Szailer

Eva Novak

Organic Synthesis with CO2 as a Reactant

A Novel Route for Carbon Dioxide Cycloaddition to Propylene Carbonate

130

(8)

W. Wei

T. Wei

Y. Sun

Catalytic Behavior of Calcium Oxide for Synthesis of Dimethyl Carbonate from Propylene Carbonate and Methanol Near Room Temperature

138

(21)

Tong Wei

M. Wang

Wei Wei

Yuhan Sun

Bin Zhong

Catalytic Esterification of Carbon Dioxide and Methanol for the Preparation of Dimethyl Carbonate

159

(10)

Fa-hai Cao

Ding-ye Fang

Dian-hua Liu

Wei-yong Ying

Electrochemical Reduction of CO2 on Cu Electrode in Methanol at Low Temperature

169

(14)

Satoshi Kaneco

Hideyuki Katsumata

Tohru Suzuki

Kiyohisa Ohta

CO2 Hydrogenation over Copper-Based Hybrid Catalysts for the Synthesis of Oxygenates

183

(12)

Son-Ki Ihm

Se-Won Baek

Young-Kwon Park

Jong-Ki Jeon

Methanol Synthesis from H2/CO/CO2 over CNT-Promoted Cu--ZnO-Al2O3 Catalyst

195

(17)

Hong-Bin Zhang

Xin Dong

Guo-Dong Lin

You-Zhu Yuan

Peng Zhang

K. R. Tsai

Biochemical Fixation of CO2

Enzymatic Conversion of Carbon Dioxide to Methanol by Dehydrogenases Encapsulated in Sol-Gel Matrix

212

(7)

Zhongyi Jiang

Hong Wu

Songwei Xu

Shufang Huang

Toward Solar Energy Conversion into Fuels: Design and Synthesis of Ruthenium--Manganese Supramolecular Complexes to Mimic the Function of Photosystem II

219

(27)

Licheng Sun

Bjorn Akermark

Leif Hammarstrom

Stenbjorn Styring

Methane Valorization

Catalytic Stability of Ni Catalyst for Partial Oxidation of Methane to Syngas

246

(14)

Zhenhua Li

Xiangyu Zhang

Fei He

Genhui Xu

Structure--Reactivity Studies of the Methane Partial Oxidation by Nitrous Oxide-Activated Iron Clusters in Various Zeolite Topologies

260

(20)

Peter-Paul H. J. M. Knops-Gerrits

Direct Partial Oxidation of Methane to Methanol in a Specially Designed Reactor

280

(12)

Qijian Zhang

Dehua He

Xin Zhang

Qiming Zhu

Shuiliang Yao

Conversion of Methane and Other Greenhouse Gases via Plasmas or Microwave Heating

Plasma Catalytic Hybrid Reforming of Methane

292

(10)

Thomas Hammer

Thomas Kappes

Wolfgang Schiene

Methane Coupling and Reforming Using Non-Equilibrium Pulsed Discharge at Room Temperature: Catalyst--Pulsed Discharge Combined System

302

(12)

S. Kado

K. Urasaki

H. Nakagawa

K. Miura

Y. Sekine

Evaluation of a High-Energy Transform Efficiency Pulse Power Supply for Methane Plasma Conversion

314

(11)

Mamoru Okumoto

Shuiliang Yao

Akira Nakayama

Eiji Suzuki

Factors Affecting the Catalytic Activation of Methane via Microwave Heating

325

(13)

L. Daniel Conde

Steven L. Suib

Decomposition of CF4 by Microwave Heating: A Potential Way to Decrease Greenhouse Gas Emissions

338

(14)

Franz-Joef Spiess

Steven L. Suib

Yuji Hayashi

Hiroshige Matsumoto

Application of Supercritical CO2

Application of High-Pressure Phase Equilibria to the Selective Oxidation of Alcohols over Supported Platinum Catalysts in Supercritical Carbon Dioxide

352

(14)

Roger Glaser

Jorg Williardt

David Bush

Michael J. Lazzaroni

Charles A. Eckert

Methane Combustion

Catalytic Combustion of Methane over Co--Mn Mixed Oxides

366

(9)

W. B. Li

Y. Lin

Y. Zhang

Supported Pd Catalyst for High-Temperature Methane Combustion: Examining the Combustion Synthesis Preparation Method

375

(12)

M. A. Fraga

M. C. Greca

L. G. Appel

Indexes

Author Index

387

(2)

Subject Index

389

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Utilization of Greenhouse Gases

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